QUROPE Quantum Information Processing and Communication in Europe

Semiconductor quantum dots are among the best sources of on-demand entangled photon pairs. The degree of entanglement, however, is generally limited by the fine structure splitting of exciton states. In this paper, we theoretically investigate the generation of polarisation-entangled photon pairs under two-photon excitation and cavity-assisted two-photon emission, both in the weak and strong cavity coupling regimes. We demonstrate and clarify that cavity coupling together with an excitation pulse reduces the degree of entanglement in three different ways. Firstly, in a strong coupling regime, cavity introduces the unequal ac-Stark shift of horizontally and vertically polarised exciton states, which results in the effective splitting of exciton states. Secondly, it induces the cross-coupling between the exciton states even in the weak coupling regime, causing the creation of unfavorable two-photon states. Finally, higher excited states of the cavity modes also contribute to the reduction of entanglement. Therefore, in the setting considered here, cavity coupling, which is generally required for the efficient collection of emitted photons, degrades the entanglement both in weak and strong coupling regimes.

We explore dissipative quantum tunnelling, a phenomenon central to various physical and chemical processes, using a double-well potential model. This paper aims to bridge gaps in understanding the crossover from thermal activation to quantum tunnelling, a domain still shrouded in mystery despite extensive research. We study a Caldeira-Leggett-derived model of quantum Brownian motion and investigate the Lindblad and stochastic Schr\"{o}dinger dynamics numerically, seeking to offer new insights into the transition states in the crossover region. Our study has implications for quantum computing and understanding fundamental natural processes, highlighting the significance of quantum effects on transition rates and temperature influences on tunnelling.

Additionally, we introduce a new model for quantum Brownian motion which takes Lindblad form and is formulated as a modification of the widely known model found in Breuer and Petruccione. In our approach, we remove the zero-temperature singularity resulting in a better description of low-temperature quantum Brownian motion near a potential minima.

We introduce an iteration-dependent scaled min-sum decoding for low-rate LDPC codes in CV-QKD, achieving near-sum product algorithm performance with reduced complexity, and facilitating CV-QKD hardware implementation.

Malware detection is an important topic of current cybersecurity, and Machine Learning appears to be one of the main considered solutions even if certain problems to generalize to new malware remain. In the aim of exploring the potential of quantum machine learning on this domain, our previous work showed that quantum neural networks do not perform well on image-based malware detection when using a few qubits. In order to enhance the performances of our quantum algorithms for malware detection using images, without increasing the resources needed in terms of qubits, we implement a new preprocessing of our dataset using Grayscale method, and we couple it with a model composed of five distributed quantum convolutional networks and a scoring function. We get an increase of around 20 \% of our results, both on the accuracy of the test and its F1-score.

To obtain spatial information about an arbitrary object in x-ray structure analysis, the standard method is to measure the intensity in the far field, i.e., the first-order photon correlation function of the coherently scattered x-ray photons (coherent diffractive imaging). Recently, it was suggested to record alternatively the incoherently scattered photons and measure the second-order photon correlation function to reconstruct the geometry of the unknown object (incoherent diffractive imaging). Yet, besides various advantages of the latter method, both techniques suffer from the so-called phase retrieval problem. Lately, an ab-initio phase retrieval algorithm to reconstruct the phase of the so-called structure factor of the scattering objects based on the third-order photon correlation function was reported. The algorithm makes use of the so-called closure phase, which contains important, yet incomplete phase information, well-known from triple correlations and their bispectrum in speckle masking and astronomy applications. Here, we provide a detailed analysis of the underlying scheme and quantities in the context of x-ray structure analysis. In particular, we explicitly calculate the third-order photon correlation function in a full quantum mechanical treatment and discuss the uniqueness of the closure phase equations constructed from it. In this context, we recapitulate the sign problem of the closure phase and how it can be lifted using redundant information. We further show how the algorithm can be improved using even higher-order photon correlation functions, e.g., the fourth-order correlation function, delivering new phase relations appearing in the four-point correlations.

The dynamics of open quantum systems connected with several reservoirs attract great attention due to its importance in quantum optics, biology, quantum thermodynamics, transport phenomena, etc. In many problems, the Born approximation is applicable which implies that the influence of the open quantum system on the reservoirs can be neglected. However, in the case of a long-time dynamics or mesoscopic reservoir, the reverse influence can be crucial. In this paper, we investigate the transient dynamics of several bosonic reservoirs connected through an open quantum system. We use an adiabatic approach to study the temporal dynamics of temperatures of the reservoirs during relaxation to thermodynamic equilibrium. We show that there are various types of temperature dynamics that strongly depend on the values of dissipative rates and initial temperatures. We demonstrate that temperatures of the reservoirs can exhibit non-monotonic behavior. Moreover, there are moments of time during which the reservoir with initially intermediate temperature becomes the hottest or coldest reservoir. The obtained results pave the way for managing energy flows in mesoscale and nanoscale systems.

We study the non-equilibrium dynamics of kicked Ising models in $1+1$ dimensions which have interactions alternating between odd and even bonds in time. These models give rise to time-evolution equivalent to quantum circuits having both the global property of tri-unitarity (three 'arrows of time') and also the local property of second-level dual-unitarity, which constrains the behavior of pairs of local gates underlying the circuit under a space-time rotation. We identify a broad class of initial product states wherein the effect of the environment on a small subsystem can be exactly represented by influence matrices with simple Markovian structures, resulting in the subsystem's full dynamics being efficiently computable. We further find additional conditions under which the dynamics of entanglement can be solved for all times, yielding rich phenomenology ranging from linear growth at half the maximal speed allowed by locality, followed by saturation to maximum entropy (i.e., thermalization to infinite temperature); to entanglement growth with saturation to extensive but sub-maximal entropy. Our findings extend our knowledge of interacting quantum systems whose thermalizing dynamics can be efficiently and analytically computed, going beyond the well-known examples of integrable models, Clifford circuits, and dual-unitary circuits.

We demonstrate continuous Pound-Drever-Hall (PDH) nondestructive monitoring of the electron spin polarization of an atomic vapor in a microfabricated vapor cell within an optical resonator. The two-chamber silicon and glass cell contains $^{87}$Rb and 1.3 amagat of N$_{2}$ buffer gas, and is placed within a planar optical resonator formed by two mirrors with dichroic dielectric coatings to resonantly enhance the coupling to phase-modulated probe light near the D$_2$ line at 780 nm. We describe the theory of signal generation in this system, including the spin-dependent complex refractive index, cavity optical transfer functions, and PDH signal response to spin polarization. We observe cavity transmission and PDH signals across $\approx 200$ GHz of detuning around the atomic resonance line. By resonant optical pumping on the 795 nm D$_1$ line, we observe spin-dependent cavity line shifts, in good agreement with theory. We use the saturation of the line shift vs. optical pumping power to calibrate the number density and efficiency of the optical pumping. In the unresolved sideband regime, we observe quantum-noise-limited PDH readout of the spin polarization density, with a flat noise floor of $9 \times 10^9$ spins cm$^{-3}$ Hz$^{-1/2}$ for frequencies above 700 Hz. We note possible extensions of the technique.

Charge-density wave phases in quantum materials stem from the complex interplay of electronic and lattice degrees of freedom. Nowadays, various time-resolved spectroscopy techniques allow to actively manipulate such phases and monitor their dynamics in real time. Modeling such nonequilibrium dynamics theoretically is a great challenge and exact methods can usually only treat a small number of atoms and finitely many phonons. We approach the melting of charge-density waves in a Holstein model after a sudden switch-on of the electronic hopping from two perspectives: We prove that in the non-interacting and in the strong-coupling limit, the CDW order parameter on high-dimensional hypercubic lattices obeys a factorization relation for long times, such that its dynamics can be reduced to the one-dimensional case. Secondly, we present numerical results from semiclassical techniques based on the Truncated Wigner Approximation for two spatial dimensions. A comparison with exact data obtained for a Holstein chain shows that a semiclassical treatment of both the electrons and phonons is required in order to correctly describe the phononic dynamics. This is confirmed, in addition, for a quench in the electron-phonon coupling strength.

We propose a theoretical project in which quantum squeezing induces quantum entanglement and Einstein-Podolsky-Rosen steering in a coupled whispering-gallery-mode optomechanical system. Through pumping the $\chi^{(2)}$-nonlinear resonator with the phase matching condition, the generated squeezed resonator mode and the mechanical mode of the optomechanical resonator can generate strong quantum entanglement and EPR steering, where the squeezing of the nonlinear resonator plays the vital role. The transitions from zero entanglement to strong entanglement and one-way steering to two-way steering can be realized by adjusting the system parameters appropriately. The photon-photon entanglement and steering between the two resonators can also be obtained by deducing the amplitude of the driving laser. Our project does not need an extraordinarily squeezed field, and it is convenient to manipulate and provides a novel and flexible avenue for diverse applications in quantum technology dependent on both optomechanical and photon-photon entanglement and steering.

During the noisy intermediate-scale quantum (NISQ) era, quantum computational approaches refined to overcome the challenge of limited quantum resources are highly valuable. However, the accuracy of the molecular properties predicted by most of the quantum computations nowadays is still far off (not within chemical accuracy) compared to their corresponding experimental data. Here, we propose a promising qubit-efficient quantum computational approach to calculate the harmonic vibrational frequencies of a large set of neutral closed-shell diatomic molecules with results in great agreement with their experimental data. To this end, we construct the accurate Hamiltonian using molecular orbitals, derived from density functional theory to account for the electron correlation and expanded in the Daubechies wavelet basis set to allow an accurate representation in real space grid points, where an optimized compact active space is further selected so that only a reduced small number of qubits is sufficient to yield an accurate result. To justify the approach, we benchmark the performance of the Hamiltonians spanned by the selected molecular orbitals by first transforming the molecular Hamiltonians into qubit Hamiltonians and then using the exact diagonalization method to calculate the results, regarded as the best results achievable by quantum computation. Furthermore, we show that the variational quantum circuit with the chemistry-inspired UCCSD ansatz can achieve the same accuracy as the exact diagonalization method except for systems whose Mayer bond order indices are larger than 2. For those systems, we demonstrate that the heuristic hardware-efficient RealAmplitudes ansatz, even with a shorter circuit depth, can provide a significant improvement over the UCCSD ansatz, verifying that the harmonic vibrational frequencies could be calculated accurately by quantum computation in the NISQ era.

Easily accessible through tabletop experiments based on laser propagation inside nonlinear optical media, Paraxial Fluids of Light are emerging as promising platforms for the simulation and exploration of quantum-like phenomena. In particular, the analogy builds on a formal equivalence between the governing model for a Bose-Einstein Condensate under the mean-field approximation and the model of laser propagation under the paraxial approximation. Yet, the fact that the role of time is played by the propagation distance in the optical analogue system may impose strong bounds on the range of accessible phenomena due to the limited length of the nonlinear medium. In this manuscript, we present a novel experimental approach to solve this limitation in the form of an optical feedback loop, which consists of the reconstruction of the optical states at the end of the system followed by their subsequent re-injection exploiting wavefront shaping techniques. The results enclosed demonstrate the potential of this approach to access unprecedented dynamics, paving for the observation of novel phenomena in these systems.

We study the performance of a quantum Otto heat engine with two spins coupled by a Heisenberg interaction, taking into account not only the mean values of work and efficiency but also their fluctuations. We first show that, for this system, the output work and its fluctuations are directly related to the magnetization and magnetic susceptibility of the system at equilibrium with either heat bath. We analyze the regions where the work extraction can be done with low relative fluctuation for a given range of temperatures, while still achieving an efficiency higher than that of a single spin system heat engine. In particular, we find that, due to the presence of `idle' levels, an increase in the inter-spin coupling can either increase or decrease fluctuations, depending on the other parameters. In all cases, however, we find that the relative fluctuations in work or efficiency remain large, implying that this microscopic engine is not very reliable as a source of work.

We report a driven-dissipative mechanism to generate stationary entangled $W$ states among strongly-interacting quantum emitters placed within a cavity. Driving the ensemble into the highest energy state -- whether coherently or incoherently -- enables a subsequent cavity-enhanced decay into an entangled steady state consisting of a single de-excitation shared coherently among all emitters, i.e., a $W$ state, well known for its robustness against qubit loss. The non-harmonic energy structure of the interacting ensemble allows this transition to be resonantly selected by the cavity, while quenching subsequent off-resonant decays. Evidence of this purely dissipative mechanism should be observable in state-of-the-art cavity QED systems in the solid-state, enabling new prospects for the scalable stabilization of quantum states in dissipative quantum platforms.

Determining the properties of molecules and materials is one of the premier applications of quantum computing. A major question in the field is how to use imperfect near-term quantum computers to solve problems of practical value. Inspired by the recently developed variants of the quantum counterpart of the equation-of-motion (qEOM) approach and the orbital-optimized variational quantum eigensolver (oo-VQE), we present a quantum algorithm (oo-VQE-qEOM) for the calculation of molecular properties by computing expectation values on a quantum computer. We perform noise-free quantum simulations of BeH$_2$ in the series of STO-3G/6-31G/6-31G* basis sets, H$_4$ and H$_2$O in 6-31G using an active space of four electrons and four spatial orbitals (8 qubits) to evaluate excitation energies, electronic absorption, and for twisted H$_4$, circular dichroism spectra. We demonstrate that the proposed algorithm can reproduce the results of conventional classical CASSCF calculations for these molecular systems.

We present the quantum simulation of the frustrated quantum spin-$\frac{1}{2}$ antiferromagnetic Heisenberg spin chain with competing nearest-neighbor $(J_1)$ and next-nearest-neighbor $(J_2)$ exchange interactions in the real superconducting quantum computer with qubits ranging up to 100. In particular, we implement, for the first time, the Hamiltonian with the next-nearest neighbor exchange interaction in conjunction with the nearest neighbor interaction on IBM's superconducting quantum computer and carry out the time evolution of the spin chain by employing first-order Trotterization. Furthermore, our novel implementation of second-order Trotterization for the isotropic Heisenberg spin chain, involving only nearest-neighbor exchange interaction, enables precise measurement of the expectation values of staggered magnetization observable across a range of up to 100 qubits. Notably, in both cases, our approach results in a constant circuit depth in each Trotter step, independent of the initial number of qubits. Our demonstration of the accurate measurement of expectation values for the large-scale quantum system using superconducting quantum computers designates the quantum utility of these devices for investigating various properties of many-body quantum systems. This will be a stepping stone to achieving the quantum advantage over classical ones in simulating quantum systems before the fault tolerance quantum era.

Information exchange between two distant parties, where information is shared without physically transporting it, is a crucial resource in future quantum networks. Doing so with high-dimensional states offers the promise of higher information capacity and improved resilience to noise, but progress to date has been limited. Here we demonstrate how a nonlinear parametric process allows for arbitrary high-dimensional state projections in the spatial degree of freedom, where a strong coherent field enhances the probability of the process. This allows us to experimentally realise quantum transport of high-dimensional spatial information facilitated by a quantum channel with a single entangled pair and a nonlinear spatial mode detector. Using sum frequency generation we upconvert one of the photons from an entangled pair resulting in high-dimensional spatial information transported to the other. We realise a d=15 quantum channel for arbitrary photonic spatial modes which we demonstrate by faithfully transferring information encoded into orbital angular momentum, Hermite-Gaussian and arbitrary spatial mode superpositions, without requiring knowledge of the state to be sent. Our demonstration merges the nascent fields of nonlinear control of structured light with quantum processes, offering a new approach to harnessing high-dimensional quantum states, and may be extended to other degrees of freedom too.

Nanodevices exploiting quantum effects are critically important elements of future quantum technologies (QT), but their real-world performance is strongly limited by decoherence arising from local `environmental' interactions. Compounding this, as devices become more complex, i.e. contain multiple functional units, the `local' environments begin to overlap, creating the possibility of environmentally mediated decoherence phenomena on new time-and-length scales. Such complex and inherently non-Markovian dynamics could present a challenge for scaling up QT, but -- on the other hand -- the ability of environments to transfer `signals' and energy might also enable sophisticated spatiotemporal coordination of inter-component processes, as is suggested to happen in biological nanomachines, like enzymes and photosynthetic proteins. Exploiting numerically exact many body methods (tensor networks) we study a fully quantum model that allows us to explore how propagating environmental dynamics can instigate and direct the evolution of spatially remote, non-interacting quantum systems. We demonstrate how energy dissipated into the environment can be remotely harvested to create transient excited/reactive states, and also identify how reorganisation triggered by system excitation can qualitatively and reversibly alter the `downstream' kinetics of a `functional' quantum system. With access to complete system-environment wave functions, we elucidate the microscopic processes underlying these phenomena, providing new insight into how they could be exploited for energy efficient quantum devices.

Quantum computers, using efficient Hamiltonian evolution routines, have the potential to simulate Green's functions of classically-intractable quantum systems. However, the decoherence errors of near-term quantum processors prohibit large evolution times, posing limits to the spectrum resolution. In this work, we show that Atomic Norm Minimization, a well-known super-resolution technique, can significantly reduce the minimum circuit depth for accurate spectrum reconstruction. We demonstrate this technique by recovering the spectral function of an impurity model from measurements of its Green's function on an IBM quantum computer. The reconstruction error with the Atomic Norm Minimization is one order of magnitude smaller than with more standard signal processing methods. Super-resolution methods can facilitate the simulation of large and previously unexplored quantum systems, and may constitute a useful non-variational tool to establish a quantum advantage in a nearer future.

We generalize the notion of quantum state designs to infinite-dimensional spaces. We first prove that, under the definition of continuous-variable (CV) state $t$-designs from Comm. Math. Phys. 326, 755 (2014), no state designs exist for $t\geq2$. Similarly, we prove that no CV unitary $t$-designs exist for $t\geq 2$. We propose an alternative definition for CV state designs, which we call rigged $t$-designs, and provide explicit constructions for $t=2$. As an application of rigged designs, we develop a design-based shadow-tomography protocol for CV states. Using energy-constrained versions of rigged designs, we define an average fidelity for CV quantum channels and relate this fidelity to the CV entanglement fidelity. As an additional result of independent interest, we establish a connection between torus $2$-designs and complete sets of mutually unbiased bases.